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At least 109 records · Page 6Linked to original sources

USGS1983

Additions of nutrients and major ions by the atmosphere and tributaries to nearshore waters of northwestern Lake Huron

Nutrient additions by the atmosphere and six tributaries to nearshore waters of northwestern Lake Huron were measured at weekly intervals from August 1975 to July 1976. The atmosphere contributed 43% of the nitrogen (N) and 10% of the phosphorus (P) that was added during the year. The 1975–76 atmospheric loading rate of total N to this area (11 kg/ha/yr) was one of the highest found to date in the United States. N was conserved more efficiently than P in the tributary drainage basins. Of the N and P that fell annually on the watersheds under study, 2 to 37% of the N and 31 to 84% of the P was carried with runoff to the lake. From a basin where ditching and clear-cutting occurred, water, P, silica (SiO 2 ), N, and sodium were lost at higher rates than from five other basins. Most of the N in bulk atmospheric samples (23%) and tributary waters (56%) was dissolved organic N, a form of N not often measured.

Michigan↗

USGS2018

Larch tree rings as a tool for reconstructing 20th century central European atmospheric mercury trends

We propose the tree rings of European Larch ( Larix decidua ) as a widely available and reliable geochemical archive of local and regional changes in atmospheric mercury (Hg). Mean Hg concentrations in larch tree rings from 8 background sites across the Czech Republic ranged from 2.2 to 4.8 μg kg –1 ; the maximum concentrations occurred in the period 1951–1970. At 3 sites impacted by Hg-emission sources [gold amalgamation processing, caustic soda production, and lead (Pb) ore smelting] mean larch tree ring Hg concentrations were significantly elevated relative to background sites. Changes in larch tree ring Hg concentrations were temporally coherent with known activities at the sites that would alter Hg emissions; the nearly simultaneous response in tree rings indicated little or no translocation of Hg within the larch bole. Based on the present-day atmospheric Hg concentration of 1.63 ng m –3 at the intensively monitored Czech Global Mercury Observation System site and the most recent mean tree ring Hg concentration of 2.8 μg kg –1 in co-located larch trees, we developed a simple distribution model of Hg between the atmosphere and larch tree rings. We applied the model using observed changes of Hg in larch tree rings from the countrywide background sites to reconstruct past atmospheric Hg concentrations in central Europe. Modeled Hg concentrations were in agreement with annual means from the European Monitoring and Evaluation Programme observatories.

Environmental Science & Technology↗

USGS2014

Decreased atmospheric sulfur deposition across the southeastern U.S.: When will watersheds release stored sulfate?

Emissions of sulfur dioxide (SO 2 ) to the atmosphere lead to atmospheric deposition of sulfate (SO 4 2- ), which is the dominant strong acid anion causing acidification of surface waters and soils in the eastern United States (U.S.). Since passage of the Clean Air Act and its Amendments, atmospheric deposition of SO 2 in this region has declined by over 80%, but few corresponding decreases in stream-water SO 4 2- concentrations have been observed in unglaciated watersheds. We calculated SO 4 2- mass balances for 27 forested, unglaciated watersheds from Pennsylvania to Georgia, by using total atmospheric deposition (wet plus dry) as input. Many of these watersheds still retain SO 4 2- , unlike their counterparts in the northeastern U.S. and southern Canada. Our analysis showed that many of these watersheds should convert from retaining to releasing SO 4 2- over the next two decades. The specific years when the watersheds crossover from retaining to releasing SO 4 2- correspond to a general geographical pattern of later net watershed release from north to south. The single most important variable that explained the crossover year was the runoff ratio, defined as the ratio of annual mean stream discharge to precipitation. Percent clay content and mean soil depth were secondary factors in predicting crossover year. The conversion of watersheds from net SO 4 2- retention to release anticipates more widespread reductions in stream-water SO 4 2- concentrations in this region.

Environmental Science & Technology↗

USGS1997

The urban atmosphere as a non-point source for the transport of MTBE and other volatile organic compounds (VOCS) to shallow groundwater

Infiltration and dispersion (including molecular diffusion) can transport volatile organic compounds (VOCs) from urban air into shallow groundwater. The gasoline additive methyl- tert -butyl ether (MTBE) is of special interest because of its (1) current levels in some urban air, (2) strong partitioning from air into water, (3) resistance to degradation, (4) use as an octane-booster since the 1970s, (5) rapidly increasing use in the 1990s to reduce CO and O 3 in urban air, and (6) its frequent detection at low microgram per liter levels in shallow urban groundwater in Denver, New England, and elsewhere. Numerical simulations were conducted using a 1-D model domain set in medium sand (depth to water table = 5 m) to provide a test of whether MTBE and other atmospheric VOCs could move to shallow groundwater within the 10−15 y time frame over which MTBE has now been used in large amounts. Degradation and sorption were assumed negligible. In case 1 (no infiltration, steady atmospheric source), 10 y was not long enough to permit significant VOC movement by diffusion into shallow groundwater. Case 2 considered a steady atmospheric source plus 36 cm/y of net infiltration; groundwater at 2 m below the water table became nearly saturated with atmospheric levels of VOC within 5 y. Case 3 was similar to case 2, but considered the source to be seasonal, being “on” for only 5 of 12 months each year, as with the use of MTBE during the winter fuel-oxygenate season; groundwater at 2 m below the water table became equilibrated with 5 / 12 of the “source-on” concentration within 5 y. Cases 4 and 5 added an evapotranspiration (ET) loss of 36 cm/y, resulting in no net recharge. Case 4 took the ET from the surface, and case 5 took the ET from the capillary fringe at a depth of 3.5 m. Net VOC mass transfer to shallow groundwater after 5 y was less for both cases 4 and 5 than for case 3. However, it was significantly greater for cases 4 and 5 than for case 1, even though cases 1, 4, and 5 were all no-net recharge cases. The mechanism responsible for this effect was the dispersion acting on each downward infiltration event, and also on the ET-induced flow. The ability of MTBE to reach groundwater in cases 2−5 is taken as evidence of the potential importance of urban air as a non-point source for VOCs in shallow urban groundwater. Two subcases were run for both case 4 and case 5: subcase a (water and VOCs move with ET) and subcase b (water only moves with ET).

Environmental Science & Technology↗

USGS2001

African desert dust in the Caribbean atmosphere: Microbiology and public health

Air samples collected on St. John in the U.S. Virgin Islands were screened for the presence of viable bacteria and fungi to determine if the number of cultivatable microbes in the atmosphere differed between "clear atmospheric conditions" and "African dust-events." Results indicate that during "African dust-events," the numbers of cultivatable airborne microorganisms can be 2 to 3 times that found during "clear atmospheric conditions." Direct microbial counts of air samples using an epifluorescent microscopy assay demonstrated that during an "African dust-event," bacteria-like and virus-like particle counts were approximately one log greater than during "clear atmospheric conditions." Bacteria-like particles exhibiting autofluoresence, a trait of phototrophs, were only detected during an "African dust-event.".

Aerobiologia↗

USGS2001

Dust in the wind: long range transport of dust in the atmosphere and its implications for global public and ecosystem health

Movement of soil particles in atmospheres is a normal planetary process. Images of Martian dust devils (wind-spouts) and dust storms captured by NASA's Pathfinder have demonstrated the significant role that storm activity plays in creating the red atmospheric haze of Mars. On Earth, desert soils moving in the atmosphere are responsible for the orange hues in brilliant sunrises and sunsets. In severe dust storm events, millions of tons of soil may be moved across great expanses of land and ocean. An emerging scientific interest in the process of soil transport in the Earth's atmosphere is in the field of public and ecosystem health. This article will address the benefits and the potential hazards associated with exposure to particle fallout as clouds of desert dust traverse the globe.

Global Change and Human Health↗

USGS2011

Exploring Martian polar atmospheric circulation and surface interactions

The northern and southern seasonal polar caps of Mars are formed in the polar night, during their respective autumn and winter seasons, by the condensation of atmospheric CO 2 directly to the solid phase as ice, snow, and possibly frost. During spring and summer, the seasonal ice sublimes, returning CO 2 to the atmosphere. The caps advance and recede in response to seasonal variations in solar insolation, extending as far as 40° from the poles, and have been noted by telescopic observers since the 17th century Roughly 25% of the atmosphere, which is 95% CO 2 by volume, is cycled into and out of the seasonal caps. The CO 2 cycle dominates atmospheric circulation on Mars, and must be thoroughly understood in order to answer fundamental questions about climate history and the global distribution of near‐surface water.

Eos, Transactions, American Geophysical Union↗

USGS2008

Climatically driven loss of calcium in steppe soil as a sink for atmospheric carbon

During the last several thousand years the semi-arid, cold climate of the Russian steppe formed highly fertile soils rich in organic carbon and calcium (classified as Chernozems in the Russian system). Analysis of archived soil samples collected in Kemannaya Steppe Preserve in 1920, 1947, 1970, and fresh samples collected in 1998 indicated that the native steppe Chernozems, however, lost 17-28 kg m-2 of calcium in the form of carbonates in 1970-1998. Here we demonstrate that the loss of calcium was caused by fundamental shift in the steppe hydrologic balance. Previously unleached soils where precipitation was less than potential evapotranspiration are now being leached due to increased precipitation and, possibly, due to decreased actual evapotranspiration. Because this region receives low levels of acidic deposition, the dissolution of carbonates involves the consumption of atmospheric CO2. Our estimates indicate that this climatically driven terrestrial sink of atmospheric CO2 is ???2.1-7.4 g C m-2 a-1. In addition to the net sink of atmospheric carbon, leaching of pedogenic carbonates significantly amplified seasonal amplitude of CO2 exchange between atmosphere and steppe soil. Copyright 2008 by the American Geophysical Union.

Global Biogeochemical Cycles↗

USGS2007

Atmospheric bromine flux from the coastal Abu Dhabi sabkhat: A ground-water mass-balance investigation

A solute mass-balance study of ground water of the 3000 km2 coastal sabkhat (salt flats) of the Emirate of Abu Dhabi, United Arab Emirates, documents an annual bromide loss of approximately 255 metric tons (0.0032 Gmoles), or 85 kg/km2. This value is an order of magnitude greater than previously published direct measurements from the atmosphere over an evaporative environment of a salar in Bolivia. Laboratory evidence, consistent with published reports, suggests that this loss is by vapor transport to the atmosphere. If this bromine flux to the atmosphere is representative of the total earth area of active salt flats then it is a significant, and generally under recognized, input to the global atmospheric bromide flux.

Geophysical Research Letters↗

USGS2012

Coupled atmosphere-ocean-wave simulations of a storm event over the Gulf of Lion and Balearic Sea

The coastal areas of the North-Western Mediterranean Sea are one of the most challenging places for ocean forecasting. This region is exposed to severe storms events that are of short duration. During these events, significant air-sea interactions, strong winds and large sea-state can have catastrophic consequences in the coastal areas. To investigate these air-sea interactions and the oceanic response to such events, we implemented the Coupled Ocean-Atmosphere-Wave-Sediment Transport Modeling System simulating a severe storm in the Mediterranean Sea that occurred in May 2010. During this event, wind speed reached up to 25 m.s-1 inducing significant sea surface cooling (up to 2°C) over the Gulf of Lion (GoL) and along the storm track, and generating surface waves with a significant height of 6 m. It is shown that the event, associated with a cyclogenesis between the Balearic Islands and the GoL, is relatively well reproduced by the coupled system. A surface heat budget analysis showed that ocean vertical mixing was a major contributor to the cooling tendency along the storm track and in the GoL where turbulent heat fluxes also played an important role. Sensitivity experiments on the ocean-atmosphere coupling suggested that the coupled system is sensitive to the momentum flux parameterization as well as air-sea and air-wave coupling. Comparisons with available atmospheric and oceanic observations showed that the use of the fully coupled system provides the most skillful simulation, illustrating the benefit of using a fully coupled ocean-atmosphere-wave model for the assessment of these storm events.

Journal of Geophysical Research↗

USGS2022

Spatial and temporal patterns in atmospheric deposition of dissolved organic carbon

Atmospheric deposition of dissolved organic carbon (DOC) to terrestrial ecosystems is a small, but rarely studied component of the global carbon (C) cycle. Emissions of volatile organic compounds (VOC) and organic particulates are the sources of atmospheric C and deposition represents a major pathway for the removal of organic C from the atmosphere. Here, we evaluate the spatial and temporal patterns of DOC deposition using 70 data sets at least one year in length ranging from 40° south to 66° north latitude. Globally, the median DOC concentration in bulk deposition was 1.7 mg L −1 . The DOC concentrations were significantly higher in tropical (<25°) latitudes compared to temperate (>25°) latitudes. DOC deposition was significantly higher in the tropics because of both higher DOC concentrations and precipitation. Using the global median or latitudinal specific DOC concentrations leads to a calculated global deposition of 202 or 295 Tg C yr −1 respectively. Many sites exhibited seasonal variability in DOC concentration. At temperate sites, DOC concentrations were higher during the growing season; at tropical sites, DOC concentrations were higher during the dry season. Thirteen of the thirty-four long-term (>10 years) data sets showed significant declines in DOC concentration over time with the others showing no significant change. Based on the magnitude and timing of the various sources of organic C to the atmosphere, biogenic VOCs likely explain the latitudinal pattern and the seasonal pattern at temperate latitudes while decreases in anthropogenic emissions are the most likely explanation for the declines in DOC concentration.

Global Biogeochemical Cycles↗

USGS1997

Equilibrium responses of global net primary production and carbon storage to doubled atmospheric carbon dioxide: Sensitivity to changes in vegetation nitrogen concentration

We ran the terrestrial ecosystem model (TEM) for the globe at 0.5° resolution for atmospheric CO 2 concentrations of 340 and 680 parts per million by volume (ppmv) to evaluate global and regional responses of net primary production (NPP) and carbon storage to elevated CO 2 for their sensitivity to changes in vegetation nitrogen concentration. At 340 ppmv, TEM estimated global NPP of 49.0 10 15 g (Pg) C yr −1 and global total carbon storage of 1701.8 Pg C; the estimate of total carbon storage does not include the carbon content of inert soil organic matter. For the reference simulation in which doubled atmospheric CO 2 was accompanied with no change in vegetation nitrogen concentration, global NPP increased 4.1 Pg C yr −1 (8.3%), and global total carbon storage increased 114.2 Pg C. To examine sensitivity in the global responses of NPP and carbon storage to decreases in the nitrogen concentration of vegetation, we compared doubled CO 2 responses of the reference TEM to simulations in which the vegetation nitrogen concentration was reduced without influencing decomposition dynamics (“lower N” simulations) and to simulations in which reductions in vegetation nitrogen concentration influence decomposition dynamics (“lower N+D” simulations). We conducted three lower N simulations and three lower N+D simulations in which we reduced the nitrogen concentration of vegetation by 7.5, 15.0, and 22.5%. In the lower N simulations, the response of global NPP to doubled atmospheric CO 2 increased approximately 2 Pg C yr −1 for each incremental 7.5% reduction in vegetation nitrogen concentration, and vegetation carbon increased approximately an additional 40 Pg C, and soil carbon increased an additional 30 Pg C, for a total carbon storage increase of approximately 70 Pg C. In the lower N+D simulations, the responses of NPP and vegetation carbon storage were relatively insensitive to differences in the reduction of nitrogen concentration, but soil carbon storage showed a large change. The insensitivity of NPP in the N+D simulations occurred because potential enhancements in NPP associated with reduced vegetation nitrogen concentration were approximately offset by lower nitrogen availability associated with the decomposition dynamics of reduced litter nitrogen concentration. For each 7.5% reduction in vegetation nitrogen concentration, soil carbon increased approximately an additional 60 Pg C, while vegetation carbon storage increased by only approximately 5 Pg C. As the reduction in vegetation nitrogen concentration gets greater in the lower N+D simulations, more of the additional carbon storage tends to become concentrated in the north temperate-boreal region in comparison to the tropics. Other studies with TEM show that elevated CO 2 more than offsets the effects of climate change to cause increased carbon storage. The results of this study indicate that carbon storage would be enhanced by the influence of changes in plant nitrogen concentration on carbon assimilation and decomposition rates. Thus changes in vegetation nitrogen concentration may have important implications for the ability of the terrestrial biosphere to mitigate increases in the atmospheric concentration of CO 2 and climate changes associated with the increases.

Global Biogeochemical Cycles↗

USGS2013

The influence of north Pacific atmospheric circulation on streamflow in the west

The annual cycle and nonseasonal variability of streamflow over western North America and Hawaii is studied in terms of atmospheric forcing elements. This study uses several decades of monthly average streamflow beginning as early as the late 1800's over a network of 38 stations. In addition to a strong annual cycle in mean streamflow and its variance at most of the stations, there is also a distinct annual cycle in the autocorrelation of anomalies that is related to the interplay between the annual cycles of temperature and precipitation. Of particular importance to these lag effects is the well-known role of water stored as snow pack, which controls the delay between peak precipitation and peak flow and also introduces persistence into the nonseasonal streamflow anomalies, with time scales from 1 month to over 1 year. The degree to which streamflow is related to winter atmospheric circulation over the North Pacific and western North America is tested using correlations with time averaged, gridded sea level pressure (SLP), which begins in 1899. Streamflow fluctuations show significant large-scale correlations for the winter (December through February) mean SLP anomaly patterns over the North Pacific with maximum correlations ranging from 0.3 to about 0.6. For streams along the west coast corridor the circulation pattern associated with positive streamflow anomalies is low pressure centered off the coast to the west or northwest, indicative of increased winter storms and an anomalous westerly-to-southwesterly wind component. For streams in the interior positive streamflow anomalies are associated with a positive SLP anomaly stationed remotely over the central North Pacific, and with negative but generally weaker SLP anomalies locally. One important influence on streamflow variability is the strength of the Aleutian Low in winter. This is represented by the familiar Pacific-North America (PNA) index and also by an index defined herein the “CNP” (Central North Pacific). This index, beginning in 1899, is taken to be the average of the SLP anomaly south of the Aleutians and the western Gulf of Alaska. Correlations between PNA or CNP and regional anomalies reflect streamflow the alternations in strength and position of the mean North Pacific storm track entering North America as well as shifts in the trade winds over the subtropical North Pacific. Regions whose streamflow is best tuned to the PNA or CNP include coastal Alaska, the northwestern United States, and Hawaii; the latter two regions have the opposite sign anomaly as the former. The pattern of streamflow variations associated with El Niño is similar, but the El Niño signal also includes a tendency for greater than normal streamflow in the southwestern United States. These indices are significantly correlated with streamflow at one to two seasons in advance of the December–August period, which may allow modestly skillful forecasts. It is important to note that streamflow variability in some areas, such as British Columbia and California, does not respond consistently to these broad scale Pacific atmospheric circulation indices, but is related to regional atmospheric anomaly features over the eastern North Pacific. Spatially, streamflow anomalies are fairly well correlated over scales of several hundred kilometers. Inspection of the spatial anomalies of stream-flow in this study suggest an asymmetry in the spatial pattern of positive versus negative streamflow anomalies in the western United States: dry patterns have tended to be larger and more spatially coherent than wet patterns.

Pacific Ocean↗

USGS2012

The influence of formation material properties on the response of water levels in wells to Earth tides and atmospheric loading

The water level in an open well can change in response to deformation of the surrounding material, either because of applied strains (tidal or tectonic) or surface loading by atmospheric pressure changes. Under conditions of no vertical fluid flow and negligible well bore storage (static-confined conditions), the sensitivities to these effects depend on the elastic properties and porosity which characterize the surrounding medium. For a poroelastic medium, high sensitivity to applied areal strains occurs for low porosity, while high sensitivity to atmospheric loading occurs for high porosity; both increase with decreasing compressibility of the solid matrix. These material properties also influence vertical fluid flow induced by areally extensive deformation and can be used to define two types of hydraulic diffusivity which govern pressure diffusion, one for applied strain and one for surface loading. The hydraulic diffusivity which governs pressure diffusion in response to surface loading is slightly smaller than that which governs fluid flow in response to applied strain. Given the static-confined response of a water well to atmospheric loading and Earth tides, the in situ drained matrix compressibility and porosity (and hence the one-dimensional specific storage) can be estimated. Analysis of the static-confined response of five wells to atmospheric loading and Earth tides gives generally reasonable estimates for material properties.

Journal of Geophysical Research Solid Earth↗

USGS1961

Isotopic composition of atmospheric hydrogen and methane

IN a recent communication, Bishop and Taylor 1 express the opinion that the tritium concentration of free hydrogen in the atmosphere has been rising over the past ten years, with a doubling time of approximately 18 months. The authors suspect that artificial tritium was released into the atmosphere several years before the Castle test series in 1954, which is commonly assumed to have led to the first pronounced rise in the tritium concentration of terrestrial surface water. Bishop and Taylor's communication includes a diagram of the logarithms of all the experimentally determined tritium values in free atmospheric hydrogen plotted against time. The plot shows that the values follow a straight line that includes the first value obtained by Faltings and Harteck 2 on atmospheric hydrogen collected in 1948.

Nature↗

USGS1992

Consumption of atmospheric methane by desert soils

Atmospheric concentrations of methane, a greenhouse gas, are increasing at a rate of about 1% yr -1 (refs 1–4). Oxidation by methylotrophic bacteria in soil is the largest terrestrial sink for atmospheric CH 4 , and is estimated to consume about 30 x 10 12 g CH 4 yr -1 (refs 4–6). Spatial and temporal variability in the rate of soil CH 4 consumption are incompletely understood 6–19 , as are the apparent inhibitory 12,13,18 or enhancing 20 effects of changes in land use. Dry deserts, which constitute 20% of total land surface, are not currently included in global soil uptake estimates. Here we describe measurements of the rate of uptake of atmospheric CH 4 by undisturbed desert soils. We observed rates as great as 4.38 mg CH 4 m -2 day -1 ; 50% of the measured rates were between 0.24 and 0.92 mg CH 4 m -2 d -1 . Uptake of CH 4 by desert soil is enhanced by rainfall after an initial soil-drainage period—opposite to the response of temperate forest soils 12 . Methane is consumed to a depth of about 2 m, allowing for deep removal of atmospheric CH 4 if near-surface conditions are unfavourable for consumption. On the basis of an annual average CH 4 consumption rate of 0.66 mg CH 4 m -2 d -1 , we estimate that the global CH 4 sink term needs to be increased by about 7 x 10 12 g yr -1 to account for the contribution of desert soils.

Nevada↗

USGS2009

Toxicity of atmospheric aerosols on marine phytoplankton

Atmospheric aerosol deposition is an important source of nutrients and trace metals to the open ocean that can enhance ocean productivity and carbon sequestration and thus influence atmospheric carbon dioxide concentrations and climate. Using aerosol samples from different back trajectories in incubation experiments with natural communities, we demonstrate that the response of phytoplankton growth to aerosol additions depends on specific components in aerosols and differs across phytoplankton species. Aerosol additions enhanced growth by releasing nitrogen and phosphorus, but not all aerosols stimulated growth. Toxic effects were observed with some aerosols, where the toxicity affected picoeukaryotes and Synechococcus but not Prochlorococcus.We suggest that the toxicity could be due to high copper concentrations in these aerosols and support this by laboratory copper toxicity tests preformed with Synechococcus cultures. However, it is possible that other elements present in the aerosols or unknown synergistic effects between these elements could have also contributed to the toxic effect. Anthropogenic emissions are increasing atmospheric copper deposition sharply, and based on coupled atmosphere-ocean calculations, we show that this deposition can potentially alter patterns of marine primary production and community structure in high aerosol, low chlorophyll areas, particularly in the Bay of Bengal and downwind of South and East Asia.

Proceedings of the National Academy of Sciences of↗

USGS2016

Observed decrease in atmospheric mercury explained by global decline in anthropogenic emissions

Observations of elemental mercury (Hg 0 ) at sites in North America and Europe show large decreases (&sim;1–2% y −1 ) from 1990 to present. Observations in background northern hemisphere air, including Mauna Loa Observatory (Hawaii) and CARIBIC (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container) aircraft flights, show weaker decreases (<1% y −1 ). These decreases are inconsistent with current global emission inventories indicating flat or increasing emissions over that period. However, the inventories have three major flaws: ( i ) they do not account for the decline in atmospheric release of Hg from commercial products; ( ii ) they are biased in their estimate of artisanal and small-scale gold mining emissions; and ( iii ) they do not properly account for the change in Hg 0 /Hg II speciation of emissions from coal-fired utilities after implementation of emission controls targeted at SO 2 and NO x . We construct an improved global emission inventory for the period 1990 to 2010 accounting for the above factors and find a 20% decrease in total Hg emissions and a 30% decrease in anthropogenic Hg 0 emissions, with much larger decreases in North America and Europe offsetting the effect of increasing emissions in Asia. Implementation of our inventory in a global 3D atmospheric Hg simulation [GEOS-Chem (Goddard Earth Observing System-Chemistry)] coupled to land and ocean reservoirs reproduces the observed large-scale trends in atmospheric Hg 0 concentrations and in Hg II wet deposition. The large trends observed in North America and Europe reflect the phase-out of Hg from commercial products as well as the cobenefit from SO 2 and NO x emission controls on coal-fired utilities.

Proceedings of the National Academy of Sciences↗