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USGS1985

U-Pb isochron age and Pb isotope systematics of the Golden Fleece vein; implications for the relationship of mineralization to the Lake City caldera, western San Juan Mountains, Colorado

A U-Pb isochron age of 27.5 + or - 0.5 m.y. has been determined for the Golden Fleece vein, southwestern Colorado, which contains an assemblage of pitchblende and gold-silver tellurides unique within the Lake City area. Initial Pb isotope ratios of ore samples from the vein ( 206 Pb/ 204 Pb = 19.08-19.58; 207 Pb/ 204 Pb = 15.643-15.682; 208 Pb/ 204 Pb = 38.533-38.84) are among the most radiogenic values reported from the San Juan Mountains and suggest that a significant component of common Pb, and possibly other metals, was derived from upper crustal Precambrian rocks by deeply circulating hydrothermal fluids. The 27.5-m.y. age of the Golden Fleece vein is identical, within analytical uncertainty, to the age of the quartz latite lavas that it cuts. This clearly documents the relationship of the vein to the waning stages of activity associated with the Uncompahgre caldera (27-29 m.y.) rather than to early activity related to the 23.1-m.y.-old Lake City caldera. Other veins in the Lake City area have Pb isotope ratios and mineral assemblages that are distinctly different from the Golden Fleece, and most of these veins are thought to be genetically related to the younger Lake City caldera.

Economic Geology↗
USGS1985

Remotely sensed limonite anomaly on Lordsburg Mesa, New Mexico: Possible implications for uranium deposits

We have identified a large, anomalously limonitic area in Cenozoic gravels on Lordsburg Mesa near Lordsburg, New Mexico, using Landsat images. Our interpretation of the geophysical and geochemical data suggests the exploration hypothesis that the Lordsburg Mesa limonite anomaly is the surface expression of a chemical trap that may contain concentrations of uranium similar to calcrete-uranium deposits. Ground water originating in the Big Burro Mountains, where uranium vein deposits are known, drains through the Lordsburg Mesa area. This ground water is apparently forced near the surface by a buried bed-rock ridge along the west side of the limonite anomaly. The resulting changes in ground-water chemistry may be precipitating uranium along the eastern margin of the limonite anomaly.

Economic Geology↗
USGS1985

xygen isotope, aeromagnetic, and gravity anomalies associated with hydrothermally altered zones in the Yankee Fork mining district, Custer County, Idaho

Epithermal Ag-Au vein and disseminated deposits in the Yankee Fork district are hosted in altered volcanic rocks having low delta 18 O values, low magnetic susceptibilities, low remanent magnetizations, and relatively high densities. These isotopic and physical quantities provide sensitive indices of rock alteration that can be contoured over areas that are much larger than zones of strong visible alteration. Such contour maps reveal a marked spatial association between the ore deposits, the steepest delta 18 O gradients, and the perimeter of zones where the rocks have extremely low total magnetizations. The oxygen isotope results indicate that the ore zones coincide with steep gradients in temperature and water/rock ratio in two fossil hydrothermal convective systems that involved fluids derived from Tertiary meteoric waters. Our magnetic measurements suggest that these same high-gradient zones also coincide with oxidation-reduction boundaries. Low aeromagnetic intensities and positive Bouguer anomalies are also associated with the altered zones in the Yankee Fork district. The intensities of these geophysical features are consistent with the size of the altered zones and with the contrast in physical properties between altered and unaltered rocks. Contour maps of the magnetic and isotopic properties of host rocks should find application in exploration for a variety of types of hydrothermal ore deposits, as well as in the study of ore controls and conditions of mineralization.

Economic Geology↗
USGS1985

Uranium mineralization in the Smith Lake district of the Grants uranium region, New Mexico.

The Mariano Lake and Ruby 1 uranium orebodies, which together comprise much of the uranium ore in the Smith Lake district of the Grants uranium region, New Mexico, occur in sandstones in the lower part of the Brushy Basin Member of the Upper Jurassic Morrison Formation. The orebodies, which are offset by faults of Laramide age, are enriched in an amorphous organic material that was introduced into the host sandstone after deposition. The enrichment by this organic material, in ore, is an important characteristic of the primary uranium deposits in the Grants uranium region. However, the close proximity of the chemically reduced ore zones to oxidized rock is suggestive that the deposits represent accumulations of uranium redistributed by reduction-oxidation processes from preexisting primary deposits.Within the ores, whole-rock abundances of organic carbon correlate positively with uranium contents. This correlation is consistent with petrologic evidence which indicates that uranium is everywhere intimately admixed with the amorphous organic material. Ore zones are also enriched in vanadium (as ore-stage vanadiferous chlorite) and sulfur (as ore-stage iron disulfide minerals with delta 34 S values ranging from -29 to -42ppm).Petrographic observations demonstrate that Smith Lake uranium mineralization occurred early (before major burial compaction) in the paragenetic sequence of host-rock diagenetic alterations but was preceded by precipitation of authigenic iron disulfides (delta 34 S values ranging from -11 to -38ppm), mixed-layered smectite-illite clays, and potassium feldspars.Additional preore alterations included dissolution of detrital sanidine and plagioclase and the leaching of iron from detrital iron-titanium oxide grains. Following mineralization, varying amounts of authigenic calcite and barite formed, both of which were partly replaced by kaolinitc. Oxidation of some previously formed iron disulfide minerals occurred late in the paragenetic sequence, as did localized precipitation of native selenium, pyrite, and very minor amounts of uranium minerals.The positive correlation between contents of uranium and organic carbon and the admixture of uranium with the amorphous organic material indicates that the Mariano Lake and Ruby 1 deposits are primary-type uranium orebodies. The offset of orebodies by Laramide faults and radiometric age determinations of the ores are also consistent with a primary origin for the deposits. Late Tertiary oxygenated ground waters locally modified original chemical and mineralogical characteristics of the ores in part by leaching some uranium. Secondary uranium minerals precipitated from the partly leached primary ores are sparse in the mine area; such recycled uranium appears to represent an insignificant proportion of the total uranium in the Smith Lake district.

Economic Geology↗
USGS1985

Mineralization of breccia pipes in northern Arizona

The Paleozoic sedimentary rocks on the Colorado Plateau of northern Arizona are host to hundreds ofbreccia pipes. The uranium and copper deposits in these breccia pipes transgress formation boundaries from the Mississippian Redwall Limestone to the Triassic Chinle Formation. They are not classic breccia pipes in that there is no volcanic rock associated with them in time or space. They are the result of solution-collapse within the Redwall Limestone and stoping of the overlying strata. The karst development in the Redwall Limestone began in the Mississippian and apparently either continued to the Triassic or was at least once again active during that time. The mineralization apparently occurred shortly thereafter, sometime during the Mesozoic. Mining activity in breccia pipes of the Grand Canyon region began during the nineteenth century and continues today with the operation of the Hack I, II, and III mines, although the exploited commodity has changed from Cu to U. Although small in size, these pipes contain samples with up to 55 percent U 3 O 8 and can yield ore averaging between 0.30 and 0.60 percent U 3 O 8 .Mineralization at the surface commonly occurs within nodules and concretions associated with pyrite and goethite and along fractures, while the primary ore of the unoxidized zones is commonly within a comminuted sandstone matrix surrounding breccia fragments of overlying formations. The ore mineral is uraninite, although associated with it are sphalerite, galena, chalcopyrite, tennantite, millerite, siegenite, and/molybdenite. Some of the surface nodules are encrusted with malachite and are exceptionally enriched in Ag. Pyrite is abundant, and the organic carbon content of some rocks is high enough to suggest that it, along with the pyrite, may be a reductant for uranium. In contrast, it is possible, if uranium were transported as a bicarbonate or carbonate complex, that only a conduit of brecciated rock was necessary to release CO 2 , thus disrupting the equilibrium and allowing uraninite to precipitate. An extensive suite of elements is significantly enriched in the mineralized rock: Ag, As, Ba, Cd, Co, Cr, Cs, Cu, Hg, Mo, Ni, Pb, Sb, Se, Sr, U, V, Zn, and the rare earth elements. Of these, Cu, Pb, Zn, Ag, and particularly As appear to be the best geochemical indicators of mineralized pipes. At present the origin of the mineralizing fluids is not known. The lack of extensive silification within the breccia, along with the 80 degrees to 173 degrees C fluid inclusion-filling temperatures on sphalerite, dolomite, quartz, and calcite, suggests relatively low-temperature mineralizing fluids, although heated in excess of what would be expected from the normal geothermal gradient on the Colorado Plateau. With the exception of the U-mineralized rock, the mineral assemblage and geochemistry is similar to Mississippi Valley-type deposits.

Economic Geology↗
USGS1985

The Schwartzwalder uranium deposit, II: Age of uranium mineralization and lead isotope constraints on genesis

U-Pb isotope analyses of ores from the Schwartzwalder uranium mine, Colorado, show that these ores have high amounts of initial (common) Pb and that the initial Pb was both variable and relatively radiogenic in its Pb isotope ratios ( 206 Pb/ 204 Pb = 26-30). As a result, the only useful approach to dating these ores is with U-Pb isochrons, and even so, some means of dealing with the variable initial Pb isotope ratios is required. Because the common Pb in these ores was apparently derived from sources of similar age and Th/U, the observed 208 Pb/ 204 Pb of these Th-free ores can be used either to identify sample suites with similar initial Pb isotope ratios or to normalize for the variable initial Pb isotope ratios. The resulting U-Pb isochrons indicate an age of mineralization for both Illinois vein and Titan vein ores of 69.3 + or - 1.1 m.y., suggesting that the deposit was formed during the earliest stages of Laramide uplift and under at least 3 km of Phanerozoic cover. The initial Pb isotope systematics of the ores show that the metals in the Schwartzwalder ores were derived from source(s) of 1,730 + or - 130-m.y.-age, with a Th/U of 2.2 + or - 0.2 and 238 U/ 204 Pb of 30 to 60. These restrictions on the source(s) of the metals rule out the possibility that the deposit could have been formed by remobilization of a Proterozoic uranium deposit, and both the 69.3-m.y.-age of the ores and their initial Pb isotope ratios preclude any contribution of metals to the deposit by younger volcanics such as those in the Denver Formation.

Economic Geology↗
USGS1985

Mineralogy, textures, and relative age relationships of massive sulfide ore in the West Shasta district, California

The Devonian massive sulfide orebodies of the West Shasta district in northern California are composed primarily of pyrite, with lesser amounts of other sulfide and gangue minerals. Examination of polished thin sections of more than 100 samples from the Mammoth, Shasta King, Early Bird, Balaklala, Keystone, and Iron Mountain mines suggests that mineralization may be divided into six paragenetic stages, the last five each separated by an episode of deformation: (1) precipitation of fine-grained, locally colloform and framboidal pyrite and sphalerite; (2) deposition of fine-grained arsenopyrite and coarse-grained pyrite, the latter enclosing tiny inclusions of pyrrhotite; (3) penetration and local replacement of sulfide minerals of stages 1 and 2 along growth zones and fractures by chalcopyrite, sphalerite, galena, ten-nantite, pyrrhotite, bornite, and idaite; (4) recrystallization and remobilization of existing minerals, locally increasing their size and euhedralism and promoting their aggregation; (5) deposition of quartz, white mica, chlorite, and calcite; and (6) formation of bornite, digenite, chalcocite, and covellite during supergene enrichment of several orebodies at the Iron Mountain mine. Despite regional greenschist facies metamorphism and local heating by intrusive bodies, enough of the original depositional features of the ore remain to suggest that the deposits in the district formed by processes similar to those that formed Kuroko- and Besshi-type massive sulfide deposits. Mineralogic and textural evidence do not support a second major episode of massive sulfide mineralization during the Permian.

Economic Geology↗
USGS1985

A reconnaissance Rb-Sr, Sm-Nd, U-Pb, and K-Ar study of some host rocks and ore minerals in the West Shasta Cu- Zn district, California

The Copley Greenstone, Balaklala Rhyolite, and Mule Mountain stock in the West Shasta Cu-Zn district, California, have Rb-Sr, Sm-Nd, U-Pb, and K-Ar systematics that indicate they are a cogenetic suite of ensimatic island-arc rocks about 400 m.y. Pervasive alteration and mineralization of these rocks, for the most part, was syngenetic and the major component of the mineralizing fluid was Devonian seawater. K-Ar ages of quartz-sericite concentrates from ore horizons and Rb-Sr systematics of a few rock and ore specimens record a later thermal and mineralizing event in the district of about 260 m.y. Contamination of some rocks with pelagic sediments is indicated by the Sm-Nd data.

Economic Geology↗
USGS1985

The plumbotectonics of the West Shasta mining district, eastern Klamath Mountains, California

The tectonic setting comprising the West Shasta mining district has often been compared with that of primitive island arcs. Concentrations of uranium, thorium, and lead and lead isotope compositions were determined for Devonian ores and rocks of the West Shasta district, eastern Klamath Mountains, California, to help evaluate the tectonic classification. The lead isotope pattern is found to be complex. From comparison of the data with those on younger ores and rocks in the region and with those isotopic patterns found in modern tectonic terranes, however, a number of conclusions are possible. A lead isotope point for the Devonian oceanic mantle is now well established from this study on the West Shasta district. This isotopic composition is in agreement with that suggested by Slawson in 1983--i.e., from a sample of massive sulfide ore from the Golinsky deposit--with a 206 Pb/ 204 Pb of 17.830, a 207 Pb/ 204 Pb of 15.450, and a 208 Pb/ 204 Pb of 37.313. If the Devonian mantle is analogous to the modern mantle, the determined value is probably at the more radiogenic end of the Devonian oceanic mantle array.Some samples of volcanic rocks and ores that have elevated values of 207 Pb/ 204 Pb and 208 Pb/ 204 Pb indicate that subducted pelagic sediments or interaction of the magmas with other sediments downsection have been involved to varying degrees in the generation of magmas. The high ratios were not attained by addition of lead to the volcanic rocks or ores during subsequent magmatic events, such as intrusion of the Permian Pit River stock to the east or of the Cretaceous Shasta Bally batholith that crops out to the south and west and may underlie part of the district. Some values of 207 Pb/ 204 Pb are sufficiently high as to suggest that West Shasta may have developed nearer a continent than was previously supposed. Lead isotope data for Quaternary volcanic rocks are somewhat more radiogenic than for Cretaceous ores and plutonic rocks. Permo-Triassic ores are again a bit less radiogenic. The isotopic differences between the Permo-Triassic and Quaternary data could be accounted for by a value for 238 U/ 204 Pb of 10.42 in common source material. Using this value of 238 U/ 204 Pb to calculate even further back to 400 m.y., the resulting ratios are found to fall very close to the "best value" for the lead isotope mixing line between the Devonian mantle and pelagic sediments. We interpret this intersection to be the "mean value" for the assimilated Devonian sediment lead--18.250 for 206 Pb/ 204 Pb and 15.582 for 207 Pb/ 204 Pb. As deduced for the lead isotope composition for the Devonian mantle at this location, the pelagic sediment, lead isotope composition also is toward the more radiogenic end of the values expected for pelagic sediments in the Devonian. Lack of sediments in the observed volcanic section of the West Shasta district suggests a submerged volcanic-arc setting (as interpreted by others for the Troodos and Samail ophiolites) rather than an island-arc situation (such as the Green Tuff area of Japan) or an incipient spreading ridge setting (that might have grown to be a subaerial Iceland). The elevated values of 207 Pb/ 204 Pb for some samples suggest a submerged volcanic are whereas the exceedingly low values of thorium--which is not easily mobilized during alteration events--for both basaltic andesites and plagiorhyolites is suggestive of depleted source material such as is found for most oceanic spreading centers. Elevated values of 207 Pb/ 204 Pb are exceedingly rare in midocean ridge basalts and low contents of thorium are known in island arcs, so a submerged volcanic arc is the preferred interpretation. Some similarity exists between the 206 Pb/ 204 Pb values of Devonian ores having elevated values of 207 Pb/ 204 Pb and those of the Permo-Triassic ores of the East Shasta district, as mentioned by Slawson in 1983. This similarity is now confirmed to be a coincidence. We find it due first of all to some incorporation of sediment lead in the magmas, followed later by some migration of radiogenic lead--probably locally derived--into the ores during subsequent events. Because there was some postdepositional lead migration into the ores, some migration of copper also into the ores cannot be excluded. Lead, especially radiogenic lead, however, is more mobile than copper. As the migrating lead is deduced to have been locally derived from the observed section rather than exotically derived, any copper added was probably locally derived also.

Economic Geology↗
USGS1985

Trace element content of gossans at four mines in the West Shasta massive sulfide district

We evaluated the trace element content of gossans at four mines in the West Shasta Cu-Zn mining district in California. We found little difference in trace element content between the chipped rock rind and whole-rock gossan samples. Gossans derived from disseminated sulfides were found to have a lower trace element content as well as a narrower range of values than did gossans derived from massive sulfides. Extreme differences in trace element concentrations in field duplicates of both chip and whole-rock gossan samples due to variations within the gossan bodies prevented use of the data at individual sampling sites for areal pattern studies. A computer program (REM), which uses a cell concept and groups the analysis of gossan at each mine, was used to characterize the trace element content. The gossan at the Mammoth mine had the highest anomaly magnitude and the highest element magnitudes for the most elements. Gossan at the Spread Eagle mine had a much different assemblage of elements relative to the other mines studied and had the lowest anomaly magnitude.

Economic Geology↗
USGS1985

Near-infrared spectra of West Shasta gossans compared with true and false gossans from Australia and Saudi Arabia

The near-infrared spectra of a suite of outcrop samples of massive sulfide gossans and false gossans representing three different weathering environments were measured and studied with X-ray, scanning electron microscope, and energy dispersive X-ray. Gossans that formed in a humid tropical environment are represented by samples from the Mt. Isa area, Queensland, Australia, and gossans that formed in an arid environment are represented by samples from several locations in Saudi Arabia. The gossans of the West Shasta massive sulfide district in California represent a weathering environment intermediate between these two extremes.On the basis of these spectral measurements, true gossans after massive sulfide deposits have spectra in the 800 to 2,500 nanometer (nm) region that are distinctly different from the spectra of false gossans. In the humid tropical environment, highly leached, newly formed kaolin minerals in the gossan cause spectral differences at about 1,400 to 2,200 nm. In the arid environment, true gossans preserve talc and minor mica from the massive sulfide deposit; these minerals are not observed in false gossans. These minerals result in spectral differences in the 2,200- to 2,300-nm region. In addition, true gossans generally have goethite spectral bands at about 900 nm as opposed to hematite spectral bands at about 850 nm for the false gossans.False gossans are not known in the West Shasta district; however, the gossan at the largest deposit, Iron Mountain, is a true gossan that has the distinctive spectral features of goethite at about 900 nm and diaspore in the 1,400- to 2,500-nm region. The other gossans also have the spectral features of goethite, but they contain a less leached mixture of kaolinite plus illite and have distinctive spectral features in the 1,400- to 2,500-nm region. These spectral differences define two groups of West Shasta gossans--inner gossans in large deposits and outer gossans at the margins of large deposits and in lesser massive sulfide deposits.

Economic Geology↗
USGS1986

A ground-water mixing model for the origin of the Imini manganese deposit (Cretaceous) of Morocco

Three beds of manganese oxide ore in a 10 m-thick dolomite unit are associated with diagenetic features, and, are accordingly also diagenetic in their present aspect. Whether primary or introduced, the Mn mineralogy is attributed to reactions between fresh and saline ground-waters as the zone of mixing passed through the dolomite unit during a period of falling sea-level. The succession of diagenetic changes is: 1) precursor carbonates, 2) dolomite-janggunite, 3) hollandite-pyrolusite-chert-calcite.-G.J.N.

Economic Geology↗
USGS1986

Rb-Sr, K-Ar, and stable isotope evidence for the ages and sources of fluid components of gold-bearing quartz veins in the northern Sierra Nevada foothills metamorphic belt, California

Gold-bearing quartz veins occur in and near major fault zones in deformed oceanic and island-arc rocks west of the main outcrop of the Sierra Nevada composite batholith. Veins typically occupy minor reverse faults that crosscut blueschist to amphibolite-grade metamorphic rocks whose metamorphic ages range from early Paleozoic to Jurassic. Vein micas and carbonate-quartz-mica assemblages that formed by hydrothermal metasomatism of ultramafic wall rocks in the Alleghany, Grass Valley, Washington, and Mother Lode districts yield concordant K-Ar and Rb-Sr ages. The dated veins are significantly younger than prograde metamorphism, penetrative deformation, and accretion of their host rocks to the continental margin. New and previously published mineralization ages from 13 localities in the Sierra foothills range from about 140 to 110 m.y. ago, with mean and median between 120 and 115 m.y. The age relations suggest that mineralizing fluids were set in motion by deep magmatic activity related to the resumption of east-dipping subduction along the western margin of North America following the Late Jurassic Nevadan collision event.CO 2 -bearing fluids responsible for metasomatism and much of the vein mica, carbonate, albite, and quartz deposition in several northern mines were isotopically heavy (delta 18 O [asymp] 8-14ppm; delta D between about -10 and -50ppm) and do not resemble seawater, magmatic, or meteoric waters. Metasomatic and vein-filling mica, dolomite, magnesite, and quartz in altered ultramafic rocks generally formed from fluids with similar Sr and O isotope ratios at a given locality. Consistent quartz-mica delta 18 O fractionations (delta 18 O (sub Q-M) = 4.5-4.9ppm) from various localities imply uniform equilibration temperatures, probably between 300 degrees and 350 degrees C. On a local (mine) scale, fluids responsible for both carbonate alteration of mafic and ultramafic wall rocks and albitic alteration of felsic and pelitic rocks had similar Sr isotope ratios.Samples from three veins in the central Alleghany district fit a 115.7 + or - 3-m.y. Rb-Sr isochron with a ( 87 Sr/ 86 Sr) i value of approximately 0.7119. Inferred 87 Sr/ 86 Sr ratios of metasomatic fluids from mines in different parts of the foothills region vary considerably (0.704-0.718), suggesting that Sr was derived from sources ranging from "western assemblage" Mesozoic ophiolitic or arc volcanic rocks to early Paleozoic continent-derived clastic rocks of the Shoo Fly Complex. Systematic geographic variations in both Sr and O isotopes can be rationalized by assuming extensive fluid interaction with rocks similar to the ones that are exposed within a few kilometers of the veins, but the ultimate sources of the fluids, and of Au and other constituents, may be independent of these. Isotopically lighter (meteoric?) fluids deposited some late quartz overgrowths and occupied secondary fluid inclusions in earlier vein quartz.

Economic Geology↗
USGS1986

A case study of soil gases as an exploration guide in glaciated terrain: Crandon massive sulfide deposit, Wisconsin

The Crandon massive sulfide deposit is covered by as much as 65 m of glacial drift. Soil gas was sampled at a depth of 0.5 m along several traverses over the deposit. Gases showing anomalies that correlate with the underlying deposit include CO 2 , CH 4 , and O 2 . CO 2 and CH 4 show positive anomalies with a background/anomaly ratio as high as 1 to 25, whereas O 2 shows negative anomalies. Oxidation of the sulfides with the production of sulfate is the probable chemical reaction producing some of the gas anomalies. The CH 4 anomalies may result from thermal cracking of hydrocarbon precursors. These results indicate that measurement of soil gases should provide a useful exploration tool in glacial terrain.

Economic Geology↗
USGS1986

Spectral reflectance of carbonatites and related alkalic igneous rocks: Selected samples from four North American localities

Laboratory spectral reflectance measurements were made in the 0.4- to 2.5-mu m wavelength range for samples collected from four North American carbonatite-alkalic igneous rock complexes. Alkalic rock spectra produced few absorption features; however, the carbonatites typically showed conspicuous carbonate, ferric and ferrous iron, and in some cases rare earth element absorption bands. Trivalent neodymium was the most abundant rare earth element producing absorption features and could be detected in amounts as low as 300 ppm. Ferrous iron was present in most dolomitic carbonatite samples and caused more intense ferrous absorption bands than commonly is seen in carbonate rocks of sedimentary origin. High carbonatite iron content also resulted in pervasive limonitic staining and related ferric iron absorption features. These absorption features sometimes masked other absorption bands.Because reflectance measurements can be carried out rapidly, with minimal sample preparation, reflectance spectroscopy may provide a useful field and laboratory tool for analyzing economic rare earth concentrations. In addition, the distinctive spectral characteristics of carbonatite material, in conjunction with the discordant spatial relationships between associated alkalic and carbonatite rocks, may provide a basis for remote-sensing detection of these complexes.

Economic Geology↗