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USGS2005

A frictional population model of seismicity rate change

We study models of seismicity rate changes caused by the application of a static stress perturbation to a population of faults and discuss our results with respect to the model proposed by Dieterich (1994). These models assume distribution of nucleation sites (e.g., faults) obeying rate-state frictional relations that fail at constant rate under tectonic loading alone, and predicts a positive static stress step at time to will cause an immediate increased seismicity rate that decays according to Omori's law. We show one way in which the Dieterich model may be constructed from simple general idead, illustratted using numerically computed synthetic seismicity and mathematical formulation. We show that seismicity rate change predicted by these models (1) depend on the particular relationship between the clock-advanced failure and fault maturity, (2) are largest for the faults closest to failure at to, (3) depend strongly on which state evolution law faults obey, and (4) are insensitive to some types of population hetrogeneity. We also find that if individual faults fail repeatedly and populations are finite, at timescales much longer than typical aftershock durations, quiescence follows at seismicity rate increase regardless of the specific frictional relations. For the examined models the quiescence duration is comparable to the ratio of stress change to stressing rate ????/??,which occurs after a time comparable to the average recurrence interval of the individual faults in the population and repeats in the absence of any new load may pertubations; this simple model may partly explain observations of repeated clustering of earthquakes. Copyright 2005 by the American Geophysical Union.

Journal of Geophysical Research B: Solid Earth↗

USGS2005

Nearshore wave-induced cyclical flexing of sea cliffs

[1] Evolution of a tectonically active coast is driven by geomorphically destructive energy supplied by ocean waves. Wave energy is episodic and concentrated; sea cliffs are battered by the geomorphic wrecking ball every 4-25 s. We measure the response of sea cliffs to wave assault by sensing the ground motion using near-coastal seismometers. Sea cliffs respond to waves in two distinct styles. High-frequency motion (20 Hz) reflects the natural frequency of the sea cliff as it rings in response to direct wave impact. Low-frequency motion in the 0.1-0.05 Hz (10-20 s) band consistently agrees with the dominant nearshore wave period. Integrating microseismic velocities suggests 50 ??m and 10 ??m displacements in horizontal and vertical directions, respectively. Displacement ellipsoids exhibit simultaneous downward and seaward sea cliff motion with each wave. Video footage corroborates the downward sea cliff flex in response to the imposed water load on the wave cut platform. Gradients in displacement amplitudes documented using multiple seismometers suggest longitudinal and shear strain of the flexing sea cliff on the order of 0.5-4 ?? strains during each wave loading cycle. As this sea cliff flexure occurs approximately 3 million times annually, it has the potential to fatigue the rock through cyclical loading. Local sea cliff retreat rates of 10 cm/yr imply that a given parcel of rock is flexed through roughly 109 cycles of increasing amplitude before exposure to direct wave attack at the cliff face. Copyright 2005 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2006

Surface drifter derived circulation in the northern and middle Adriatic Sea: Response to wind regime and season

More than 120 satellite-tracked drifters were deployed in the northern and middle Adriatic (NMA) Sea between September 2002 and November 2003, with the purpose of studying the surface circulation at mesoscale to seasonal scale in relation to wind forcing, river runoff, and bottom topography. Pseudo-Eulerian and Lagrangian statistics were calculated from the low-pass-filtered drifter velocity data between September 2002 and December 2003. The structure of the mean circulation is determined with unprecedented high horizontal resolution by the new data. In particular, mean currents, velocity variance, and kinetic energy levels are shown to be maximal in the Western Adriatic Current (WAC). Separating data into seasons, we found that the mean kinetic energy is maximal in fall, with high values also in winter, while it is significantly weaker in summer. High-resolution Local Area Model Italy winds were used to relate the drifter velocities to the wind fields. The surface currents appear to be significantly influenced by the winds. The mean flow during the northeasterly bora regime shows an intensification of the across-basin recirculating currents. In addition, the WAC is strongly intensified both in intensity and in its offshore lateral extension. In the southeasterly sirocco regime, northward flow without recirculation dominates in the eastern half of the basin, while during northwesterly maestro the WAC is enhanced. Separating the data into low and high Po River discharge rates for low-wind conditions shows that the WAC and the velocity fluctuations in front of the Po delta are stronger for high Po River runoff. Lagrangian covariance, diffusivity, and integral time and space scales are larger in the along-basin direction and are maximal in the southern portion of the WAC. Copyright 2006 by the American Geophysical Union.

Journal of Geophysical Research C: Oceans↗

USGS2008

Northerly surface winds over the eastern North Pacific Ocean in spring and summer

Persistent spring and summer northerly surface winds are the defining climatological feature of the western coast of North America, especially south of the Oregon coast. Northerly surface winds are important for upwelling and a vast array of other biological, oceanic, and atmospheric processes. Intermittence in northerly coastal surface wind is characterized and wind events are quantitatively defined using coastal buoy data south of Cape Mendocino on the northern California coast. The defined wind events are then used as a basis for composites in order to explain the spatial evolution of various atmospheric and oceanic processes. Wind events involve large-scale changes in the three-dimensional atmospheric circulation including the eastern North Pacific subtropical anticyclone and southeast trade winds. Composites of QSCAT satellite scatterometer wind estimates from 1999 to 2005 based on a single coastal buoy indicate that wind events typically last 72-96 h and result in anomalies in surface wind and Ekman pumping that extend over 1000 kin from the west coast of North America. It may be useful to consider ocean circulation and dependent ecosystem dynamics and the distribution of temperature, moisture, and aerosols in the atmospheric boundary layer in the context of wind events defined herein. Copyright 2008 by the American Geophysical Union.

Journal of Geophysical Research D: Atmospheres↗

USGS2008

In situ Raman spectroscopic investigation of the structure of subduction-zone fluids

In situ Raman spectra of synthetic subduction-zone fluids (KAlSi3O8-H2O system) were measured to 900?? and 2.3 GPa using a hydrothermal diamond-anvil cell. The structures of aqueous fluid and hydrous melt become closer when conditions approach the second critical endpoint. Almost no three-dimensional network was observed in the supercritical fluid above 2 GPa although a large amount of silicate component is dissolved, suggesting that the physical and chemical properties of these phases change drastically at around the second critical endpoint. Our experimental results indicate that the fluids released from a subducting slab change from aqueous fluid to supercritical fluid with increasing depth under the volcanic arcs. Copyright 2008 by the American Geophysical Union.

Journal of Geophysical Research B: Solid Earth↗

USGS2008

Magnetic fabric of sheared till: A strain indicator for evaluating the bed deformation model of glacier flow

Wet-based portions of ice sheets may move primarily by shearing their till beds, resting in high sediment fluxes and the development of subglacial landforms. This model of glacier movement, which requires high bed shear strains, can be tested using till microstructural characteristics that evolve during till deformation. Here we examine the development of magnetic fabric using a ring shear device to defom two Wisconsin-age basal tills to shear strains as high as 70. Hysteresis experiments and the dependence of magnetic susceptibility of these tills on temperature demonstrate that anisotropy of magnetic susceptibility (AMS) develops during shear due to the rotation of primarily magnetite particles that are silt sized or smaller. At moderate shear strains (???6-25), principal axes of maximum magnetic susceptibility develop a strong fabric (S1 eignevalues of 0.83-0.96), without further strengthening at higher strains, During deformation, directions of maximum susceptibility cluster strongly in the direction of shear and plunge 'up-glacier,' consistent with the behavior of pebbles and sand particles studied in earlier experiments. In contrast, the magnitude of AMS does not vary systematically with strain and is small relative to its variability among samples; this is because most magnetite grains are contained as inclusions in larger particles and hence do not align during shear. Although processes other than pervasive bed deformation may result in strong flow parallel fabrics, AMS fabrics provide a rapid and objective means of identifying basal tills that have not been sheared sufficiently to be compatible with the bed deformation model. Copyright 2008 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2009

Rupture parameters of the 2003 Zemmouri (M w 6.8), Algeria, earthquake from joint inversion of interferometric synthetic aperture radar, coastal uplift, and GPS

We study the surface deformation associated with the 21 May 2003 (M w = 6.8) Zemmouri (Algeria) earthquake, the strongest seismic event felt in the Algiers region since 1716. The thrust earthquake mechanism and related surface deformation revealed an average 0.50 m coastal uplift along ??55-km-long coastline. We obtain coseismic interferograms using Envisat advanced synthetic aperture radar (ASAR) (IS2) and RADARSAT standard beam (ST4) data from both the ascending and descending orbits of Envisat satellite, whereas the RADARSAT data proved useful only in the descending mode. While the two RADARSAT interferograms cover the earthquake area, Envisat data cover only the western half of the rupture zone. Although the interferometric synthetic aperture radar (InSAR) coherence in the epicenter area is poor, deformation fringes are observed along the coast in different patches. In the Boumerdes area, the maximum coseismic deformation is indicated by the high gradient of fringes visible in all interferograms in agreement with field measurements (tape, differential GPS, leveling, and GPS). To constrain the earthquake rupture parameters, we model the interferograms and uplift measurements using elastic dislocations on triangular fault patches in an elastic and homogeneous half-space. We invert the coseismic slip using first, a planar surface and second, a curved fault, both constructed from triangular elements using Poly3Dinv program that uses a damped least square minimization. The best fit of InSAR, coastal uplift, and GPS data corresponds to a 65-km-long fault rupture dipping 40?? to 50?? SE, located at 8 to 13 km offshore with a change in strike west of Boumerdes from N60??-65?? to N95??-105??. The inferred rupture geometry at depth correlates well with the seismological results and may have critical implications for the seismic hazard assessment of the Algiers region. Copyright 2009 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2009

Moon meteoritic seismic hum: Steady state prediction

We use three different statistical models describing the frequency of meteoroid impacts on Earth to estimate the seismic background noise due to impacts on the lunar surface. Because of diffraction, seismic events on the Moon are typically characterized by long codas, lasting 1 h or more. We find that the small but frequent impacts generate seismic signals whose codas overlap in time, resulting in a permanent seismic noise that we term the "lunar hum" by analogy with the Earth's continuous seismic background seismic hum. We find that the Apollo era impact detection rates and amplitudes are well explained by a model that parameterizes (1) the net seismic impulse due to the impactor and resulting ejecta and (2) the effects of diffraction and attenuation. The formulation permits the calculation of a composite waveform at any point on the Moon due to simulated impacts at any epicentral distance. The root-mean-square amplitude of this waveform yields a background noise level that is about 100 times lower than the resolution of the Apollo long-period seismometers. At 2 s periods, this noise level is more than 1000 times lower than the low noise model prediction for Earth's microseismic noise. Sufficiently sensitive seismometers will allow the future detection of several impacts per day at body wave frequencies. Copyright 2009 by the American Geophysical Union.

Journal of Geophysical Research E: Planets↗

USGS1998

Nonlinear refraction and reflection travel time tomography

We develop a rapid nonlinear travel time tomography method that simultaneously inverts refraction and reflection travel times on a regular velocity grid. For travel time and ray path calculations, we apply a wave front method employing graph theory. The first-arrival refraction travel times are calculated on the basis of cell velocities, and the later refraction and reflection travel times are computed using both cell velocities and given interfaces. We solve a regularized nonlinear inverse problem. A Laplacian operator is applied to regularize the model parameters (cell slownesses and reflector geometry) so that the inverse problem is valid for a continuum. The travel times are also regularized such that we invert travel time curves rather than travel time points. A conjugate gradient method is applied to minimize the nonlinear objective function. After obtaining a solution, we perform nonlinear Monte Carlo inversions for uncertainty analysis and compute the posterior model covariance. In numerical experiments, we demonstrate that combining the first arrival refraction travel times with later reflection travel times can better reconstruct the velocity field as well as the reflector geometry. This combination is particularly important for modeling crustal structures where large velocity variations occur in the upper crust. We apply this approach to model the crustal structure of the California Borderland using ocean bottom seismometer and land data collected during the Los Angeles Region Seismic Experiment along two marine survey lines. Details of our image include a high-velocity zone under the Catalina Ridge, but a smooth gradient zone between. Catalina Ridge and San Clemente Ridge. The Moho depth is about 22 km with lateral variations. Copyright 1998 by the American Geophysical Union.

Journal of Geophysical Research B: Solid Earth↗

USGS2000

Synthetic aperture radar interferometry of Okmok volcano, Alaska: radar observations

ERS-1/ERS-2 synthetic aperture radar interferometry was used to study the 1997 eruption of Okmok volcano in Alaska. First, we derived an accurate digital elevation model (DEM) using a tandem ERS-1/ERS-2 image pair and the preexisting DEM. Second, by studying changes in interferometric coherence we found that the newly erupted lava lost radar coherence for 5-17 months after the eruption. This suggests changes in the surface backscattering characteristics and was probably related to cooling and compaction processes. Third, the atmospheric delay anomalies in the deformation interferograms were quantitatively assessed. Atmospheric delay anomalies in some of the interferograms were significant and consistently smaller than one to two fringes in magnitude. For this reason, repeat observations are important to confidently interpret small geophysical signals related to volcanic activities. Finally, using two-pass differential interferometry, we analyzed the preemptive inflation, coeruptive deflation, and posteruptive inflation and confirmed the observations using independent image pairs. We observed more than 140 cm of subsidence associated with the 1997 eruption. This subsidence occurred between 16 months before the eruption and 5 months after the eruption, was preceded by ∼18 cm of uplift between 1992 and 1995 centered in the same location, and was followed by ∼10 cm of uplift between September 1997 and 1998. The best fitting model suggests the magma reservoir resided at 2.7 km depth beneath the center of the caldera, which was ∼5 km from the eruptive vent. We estimated the volume of the erupted material to be 0.055 km 3 and the average thickness of the erupted lava to be ∼7.4 m. Copyright 2000 by the American Geophysical Union.

Journal of Geophysical Research B: Solid Earth↗

USGS2005

An efficient algorithm for double-difference tomography and location in heterogeneous media, with an application to the Kilauea volcano

Improving our understanding of crustal processes requires a better knowledge of the geometry and the position of geological bodies. In this study we have designed a method based upon double-difference relocation and tomography to image, as accurately as possible, a heterogeneous medium containing seismogenic objects. Our approach consisted not only of incorporating double difference in tomography but also partly in revisiting tomographic schemes for choosing accurate and stable numerical strategies, adapted to the use of cross-spectral time delays. We used a finite difference solution to the eikonal equation for travel time computation and a Tarantola-Valette approach for both the classical and double-difference three-dimensional tomographic inversion to find accurate earthquake locations and seismic velocity estimates. We estimated efficiently the square root of the inverse model's covariance matrix in the case of a Gaussian correlation function. It allows the use of correlation length and a priori model variance criteria to determine the optimal solution. Double-difference relocation of similar earthquakes is performed in the optimal velocity model, making absolute and relative locations less biased by the velocity model. Double-difference tomography is achieved by using high-accuracy time delay measurements. These algorithms have been applied to earthquake data recorded in the vicinity of Kilauea and Mauna Loa volcanoes for imaging the volcanic structures. Stable and detailed velocity models are obtained: the regional tomography unambiguously highlights the structure of the island of Hawaii and the double-difference tomography shows a detailed image of the southern Kilauea caldera-upper east rift zone magmatic complex. Copyright 2005 by the American Geophysical Union.

Hawaii↗

USGS2006

Influence of a dam on fine-sediment storage in a canyon river

Glen Canyon Dam has caused a fundamental change in the distribution of fine sediment storage in the 99-km reach of the Colorado River in Marble Canyon, Grand Canyon National Park, Arizona. The two major storage sites for fine sediment (i.e., sand and finer material) in this canyon river are lateral recirculation eddies and the main-channel bed. We use a combination of methods, including direct measurement of sediment storage change, measurements of sediment flux, and comparison of the grain size of sediment found in different storage sites relative to the supply and that in transport, in order to evaluate the change in both the volume and location of sediment storage. The analysis shows that the bed of the main channel was an important storage environment for fine sediment in the predam era. In years of large seasonal accumulation, approximately 50% of the fine sediment supplied to the reach from upstream sources was stored on the main-channel bed. In contrast, sediment budgets constructed for two short-duration, high experimental releases from Glen Canyon Dam indicate that approximately 90% of the sediment discharge from the reach during each release was derived from eddy storage, rather than from sandy deposits on the main-channel bed. These results indicate that the majority of the fine sediment in Marble Canyon is now stored in eddies, even though they occupy a small percentage (???17%) of the total river area. Because of a 95% reduction in the supply of fine sediment to Marble Canyon, future high releases without significant input of tributary sediment will potentially erode sediment from long-term eddy storage, resulting in continued degradation in Marble Canyon. Copyright 2006 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2005

Coseismic slip distribution of the 1923 Kanto earthquake, Japan

The slip distribution associated with the 1923 M = 7.9 Kanto, Japan, earthquake is reexamined in light of new data and modeling. We utilize a combination of first-order triangulation, second-order triangulation, and leveling data in order to constrain the coseismic deformation. The second-order triangulation data, which have not been utilized in previous studies of 1923 coseismic deformation, are associated with only slightly smaller errors than the first-order triangulation data and expand the available triangulation data set by about a factor of 10. Interpretation of these data in terms of uniform-slip models in a companion study by Nyst et al. shows that a model involving uniform coseismic slip on two distinct rupture planes explains the data very well and matches or exceeds the fit obtained by previous studies, even one which involved distributed slip. Using the geometry of the Nyst et al. two-plane slip model, we perform inversions of the same geodetic data set for distributed slip. Our preferred model of distributed slip on the Philippine Sea plate interface has a moment magnitude of 7.86. We find slip maxima of ???8-9 m beneath Odawara and ???7-8 m beneath the Miura peninsula, with a roughly 2:1 ratio of strike-slip to dip-slip motion, in agreement with a previous study. However, the Miura slip maximum is imaged as a more broadly extended feature in our study, with the high-slip region continuing from the Miura peninsula to the southern Boso peninsula region. The second-order triangulation data provide good evidence for ???3 m right-lateral strike slip on a 35-km-long splay structure occupying the volume between the upper surface of the descending Philippine Sea plate and the southern Boso peninsula. Copyright 2005 by the American Geophysical Union.

Journal of Geophysical Research B: Solid Earth↗

USGS2005

Flow strength of highly hydrated Mg- and Na-sulfate hydrate salts, pure and in mixtures with water ice, with application to Europa

We selected two Europan-ice-shell candidate highly hydrated sulfate salts for a laboratory survey of ductile flow properties: MgSO4 ?? 7H2O (epsomite) and Na2SO4 ?? 10H2O (mirabilite), called MS7 and NS10, respectively. Polycrystalline samples in pure form and in mixtures with water ice I were tested using our cryogenic high-pressure creep apparatus at temperatures 232 ??? T ??? 294 K, confining pressures P = 50 and 100 MPa, and strain rates 4 ?? 10-8 ??? ???dot;e ??? 7 ?? 10-5 s-1. Grain size of NS10 samples was > 100 ??m. The flow strength ?? of pure MS7 was over 100 times that of polycrystalline ice I at comparable conditions; that of pure NS10 over 20 times that of ice. In terms of the creep law ???dot;e = A??n e-Q/RT, where R is the gas constant, we determine parameter values of A = 1012.1 MPa-ns-1, n = 5.4, and Q = 128 kJ/mol for pure NS10. Composites of ice I and NS10 of volume fraction ?? NS10 have flow strength ??c = [??NS10??NS10J + (1 - ?? NS10)??iceIJ]1/J where J ??? -0.5, making the effect on the flow of ice with low volume fractions of NS10 much like that of virtually undeformable hard rock inclusions. Being much stronger and denser than ice, massive sulfate inclusions in the warmer, ductile layer of the Europan ice shell are less likely to be entrained in convective ice flow and more likely to be drawn to the base of the ice shell by gravitational forces and eventually expelled. With only smaller, dispersed sulfate inclusions, at probable sulfate ?? < 0.2, the shell may be treated rheologically as pure, polycrystalline ice, with boundary conditions perhaps influenced by the high density and low thermal conductivity of the hydrated salts. Copyright 2005 by the American Geophysical Union.

Journal of Geophysical Research E: Planets↗

USGS2005

Evolving force balance at Columbia Glacier, Alaska, during its rapid retreat

Changes in driving and resistive stresses play an essential role in governing the buoyancy forces that are important controls on the speed and irreversibility of tidewater glacier retreats. We describe changes in geometry, velocity, and strain rate and present a top-down force balance analysis performed over the lower reach of Columbia Glacier. Our analysis uses new measurements and estimates of basal topography and photogrammetric surface velocity measurements made between 1977 and 2001, while assuming depth-independent strain. Sensitivity tests show that the method is robust and insensitive to small changes in the calculation parameters. Spatial distributions of ice speed show little correspondence with driving stress. Instead, spatial patterns of ice speed exhibit a nonlinear correspondence with basal drag. Primary resistance to flow comes from basal drag, but lateral drag becomes increasingly more important throughout the retreat, which may account for observed increases in speed. Maximum basal drag is always located in a prominent constriction located ~12 km upstream from the preretreat terminus. Once the terminus retreated into deep water off the terminal moraine marking the modern maximum extent, the upstream location of this maximum basal drag helped to promote thinning and decrease effective pressure in the lower region by limiting replenishing ice flow from upstream. An increase in both ice velocity and calving resulted, initiating what appears to be an irreversible retreat. Copyright 2005 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2007

Geochemical evidence for African dust inputs to soils of western Atlantic islands: Barbados, the Bahamas, and Florida

We studied soils on high-purity limestones of Quaternary age on the western Atlantic Ocean islands of Barbados, the Florida Keys, and the Bahamas. Potential soil parent materials in this region, external to the carbonate substrate, include volcanic ash from the island of St. Vincent (near Barbados), volcanic ash from the islands of Dominica and St. Lucia (somewhat farther from Barbados), the fine-grained component of distal loess from the lower Mississippi River Valley, and wind-transported dust from Africa. These four parent materials can be differentiated using trace elements (Sc, Cr, Th, and Zr) and rare earth elements that have minimal mobility in the soil-forming environment. Barbados soils have compositions that indicate a complex derivation. Volcanic ash from the island of St. Vincent appears to have been the most important influence, but African dust is a significant contributor, and even Mississippi River valley loess may be a very minor contributor to Barbados soils. Soils on the Florida Keys and islands in the Bahamas appear to have developed mostly from African dust, but Mississippi River valley loess may be a significant contributor. Our results indicate that inputs of African dust are more important to the genesis of soils on islands in the western Atlantic Ocean than previously supposed. We hypothesize that African dust may also be a major contributor to soils on other islands of the Caribbean and to soils in northern South America, central America, Mexico, and the southeastern United States. Dust inputs to subtropical and tropical soils in this region increase both nutrient-holding capacity and nutrient status and thus may be critical in sustaining vegetation. Copyright 2007 by the American Geophysical Union.

Journal of Geophysical Research F: Earth Surface↗

USGS2008

Surface albedo observations at Gusev Crater and Meridiani Planum, Mars

During the Mars Exploration Rover mission, the Pancam instrument has periodically acquired large-scale panoramic images with its broadband (739??338 nm) filter in order to estimate the Lambert bolometric albedo of the surface along each rover's traverse. In this work we present the full suite of such estimated albedo values measured to date by the Spirit and Opportunity rovers along their traverses in Gusev Crater and Meridiani Planum, respectively. We include estimated bolometric albedo values of individual surface features (e.g., outcrops, dusty plains, aeolian bed forms, wheel tracks, light-toned soils, and crater walls) as well as overall surface averages of the 43 total panoramic albedo data sets acquired to date. We also present comparisons to estimated Lambert albedo values taken from the Mars Global Surveyor Mars Orbiter Camera (MOC) along the rovers' traverses, and to the large-scale bolometric albedos of the sites from the Viking Orbiter Infrared Thermal Mapper (IRTM) and Mars Global Surveyor/Thermal Emission Spectrometer (TES). The ranges of Pancam-derived albedos at Gusev Crater (0.14 to 0.25) and in Meridiani Planum. (0.10 to 0.18) are in good agreement with IRTM, TES, and MOC orbital measurements. These data sets will be a useful tool and benchmark for future investigations of albodo variations with time, including measurements from orbital instruments like the Context Camera and High Resolution Imaging Science Experiment on Mars Reconnaissance Orbiter. Long-term, accurate albedo measurements could also be important for future efforts in climate modeling as well as for studies of active surface processes. Copyright 2008 by the American Geophysical Union.

Journal of Geophysical Research E: Planets↗

USGS2008

Oceanic loading of wildfire-derived organic compounds from a small mountainous river

Small mountainous rivers (SMRs) export substantial amounts of sediment into the world's oceans. The concomitant yield of organic carbon (OC) associated with this class of rivers has also been shown to be significant and compositionally unique. We report here excessively high loadings of polycyclic aromatic hydrocarbons (PAHs), lignin, and levoglucosan, discharged from the Santa Clara River into the Santa Barbara Channel. The abundance of PAHs, levoglucosan, and lignin in Santa Barbara Channel sediments ranged from 201.7 to 1232.3 ng gdw-1, 1.3 to 6.9 ??g gdw-1, and 0.3 to 2.2 mg per 100 mg of the sedimentary OC, respectively. Assuming a constant rate of sediment accumulation, the annual fluxes of PAHs, levoglucosan, and lignin, to the Santa Barbara Channel were respectively, 885.5 ?? 170.2 ng cm-2 a-1, 3.5 ?? 1.9 ??g cm-2 a-1 and 1.4 ?? 0.3 mg per 100 mg OC cm-2 a-1, over ???30 years. The close agreement between PAHs, levoglucosan, and lignin abundance suggests that the depositional flux of these compounds is largely biomass combustion-derived. To that end, use of the Santa Clara River as a model for SMRs suggests this class of rivers may be one of the largest contributors of pyrolyzed carbon to coastal systems and the open ocean. Wildfire associated carbon discharged from other high yield fluvial systems, when considered collectively, may be a significant source of lignin, pyrolytic PAHs, and other pyrogenic compounds to the ocean. Extrapolating these methods over geologic time may offer useful historical information about carbon sequestration and burial in coastal sediments and affect coastal carbon budgets. Copyright 2008 by the American Geophysical Union.

Journal of Geophysical Research G: Biogeosciences↗