Geology topics

Carl Lamborg

Publications and source records attributed to Carl Lamborg.

3 recordsLinked to original sources

USGS2026

Mercury mobilization and export from the Greenland Ice Sheet using an ice-to-ocean approach

The Greenland Ice Sheet (GrIS) is a poorly constrained source of mercury (Hg) to Arctic ecosystems. We measured Hg concentrations and stable isotopes along an ice-to-ocean continuum to identify controls on GrIS Hg export. Early-season permafrost melt and rainfall produced high filtered total mercury (fTHg, ~17 pM) and monomethylmercury (MMHg, ~2 pM). As subglacial drainage evolved, particulate Hg doubled (from ~8 to 17 pM) and MMHg production remained elevated, indicating Hg mobilization from subglacial environments. Shifts in Hg stable isotope ratios and Δ 199 Hg mass balance show supraglacial sources contribute 20–48% of exported Hg, suggesting subglacial inputs dominate the seasonal Hg flux. Fjord waters were enriched in fTHg ( ~ 10 pM) and MMHg ( ~ 2 pM) relative to rivers, consistent with particulate Hg transformations and terrestrial Hg inputs. The estimated GrIS Hg yield ( ~ 23 mmol km −2 yr −1 ) is similar to that of Arctic rivers and will likely increase with climate-driven mass loss.

Communications Earth & Environment↗

USGS2019

Mercury speciation and retention in a salt marsh undergoing long-term fertilization

Experimental plots in Great Sippewissett Marsh (Falmouth, MA USA) have been undergoing long-term (>48 years) fertilization through the application of commercial sewage sludge-based fertilizer. The experimental treatment focuses on the effect of added nitrogen on the salt marsh plots, but also supplies mercury (Hg) and other metals. This experiment provides a unique opportunity to test hypotheses regarding the Hg-related response of coastal marine ecosystems to eutrophication as well as assess the efficacy of salt marshes as sinks for increased loadings of Hg to the coastal zone. Hg inventories in sediments of control plots were similar to loadings from atmospheric deposition and inventories in the fertilized plots closely reflected the estimated loadings of Hg contained in the added fertilizer. In both the control and fertilized plots, distribution of Hg appeared somewhat different than the history of loadings, implying some level of Hg mobility. The relative abundance of monomethylmercury (CH 3 Hg + ) within the plots varied with the amount of fertilizer applied with the highest percentage of Hg as CH 3 Hg + found in the control plots, and the lowest percentages of CH 3 Hg + and S were measured in plots fertilized at the highest dose. The results from this marsh suggest that eutrophication indirectly lowers CH 3 Hg + production in this particular ecosystem, but perhaps not as a result of the sequestration of Hg(II) with S.

Estuarine, Coastal and Shelf Science↗

USGS2018

Global and local sources of mercury deposition in coastal New England reconstructed from a multi-proxy, high-resolution, estuarine sediment record

Historical reconstruction of mercury (Hg) accumulation in natural archives, especially lake sediments, has been essential to understanding human perturbation of the global Hg cycle. Here we present a high-resolution chronology of Hg accumulation between 1727 and 1996 in a varved sediment core from the Pettaquamscutt River Estuary (PRE), Rhode Island. Mercury accumulation is examined relative to (1) historic deposition of polycyclic aromatic hydrocarbons (PAHs) and lead (Pb) and its isotopes ( 206 Pb/ 207 Pb) in the same core, and (2) other reconstructions of Hg deposition in urban and remote settings. Mercury deposition in PRE parallels the temporal patterns of PAHs, and both track industrialization and regional coal use between 1850 and 1950 as well as rising petroleum use after 1950. There is little indication of increased Hg deposition from late 19th-century silver and gold mining in the western U.S. A broad maximum of Hg deposition during 1930–1980, and not found in remote sites, is consistent with the predicted influence of additional industrial sources and commercial products. Our results imply that a significant portion of global anthropogenic Hg emissions during the 20th century was deposited locally, near urban and industrial centers of Hg use and release.

Connecticut, Maine, New Hampshire, Massachusetts, ↗